Two unmet clinical needs facing the management of prostate cancer are to determine the best treatment for individual patients and to evaluate therapy response. In this study, we applied 3D dynamic imaging technique using hyperpolarized 13C nuclei to non-invasively probe prostate cancer metabolism. Pyruvate-to-lactate conversion kPL correlated well with biopsy and histological finding in pre-surgery prostate cancer patients. kPL values dramatically decreased in a patient 6 weeks into androgen-deprivation therapy with associated PSA decrease, indicating early treatment response. A non-responder patient with castration-resistant cancer exhibited high kPL one month after treatment that correlated with clinical progression.
Sequences: A 3D dynamic compressed-sensing EPSI (3D CS-EPSI) sequence was developed and translated to provide full coverage of the human prostate gland with 8x8x8mm isotropic resolution (0.5cc voxel)8,9 using a clamshell volume coil for RF transmit and endorectal coil for reception. A variable RF flip angle scheme was designed to provide constant pyruvate while maximizing lactate signal10. The RF pulses also featured reduced peak power and B1+ insensitivity for reliability in patient studies11. Some sequence parameters include: TE/TR = 4.0/150ms, temporal resolution = 2s, FOV = 9.6x9.6x12.8cm. The exams included the standard multiparametric-MRI protocol with T2-weighted images for anatomic reference12.
HP-13C MRI experiments: Following polarization in a 5T Spinlab polarizer for 2.5-3 hours, dissolutions yielded 235±15 mM sterile pyruvate with 41±6% polarization, 0.8±0.3uM radical and 32.1±0.6°C temperature that met all safety and sterility criteria prior to pharmacist release. The bolus was delivered through the antecubital vein with 0.43ml/kg dosage and injection rate of 5ml/s. All human studies were approved by the Internal Review Board at UCSF.
The first patient presented with biopsy-proven prostate cancer of Gleason score 4+5, 4+4 and 4+3 involving the majority of the left lobe, extending into the right peripheral zone with MR stage T3b and a PI-RADs score of 5. The 3D dynamic CS-EPSI sequence provided coverage of the entire prostate gland base to apex with 8mm isotropic resolution (Fig.1A). The HP-13C pyruvate bolus arrived at the vasculature around rectum, and into the prostate ~20 seconds after the end of injection. Spectroscopy data was extracted from each voxel, and pyruvate-lactate conversion rate kPL was evaluated based on two-site exchange model fit. kPL was found to be 0.02-0.04s-1 in regions of cancer (Fig.1B).
High kPL was found at regions that correlated with biopsy finding of the cancer, and lesion on the T2w images as a well-defined lesion of low signal intensity, and also regions with restricted diffusion on high b-value ADC maps (Fig.2A). Ga-68 PSMA PET-CT images were acquired at the time of mp-MRI studies (Fig.2B), showing lymph node and bone metastases (red and yellow arrows). The HP-13C MRI and PET-CT provides complementary information where the former shows the metabolism in primary prostate cancer, whereas the latter picks up metastasis.
The same patient underwent ADT (Lupron+Casodex) and chemo (docetaxel) therapies after the baseline study. Follow-up exam conducted 6 weeks after the initiation of treatment revealed markedly reduced kPL across the entire tumor region to ~1/4 compared to baseline (0.0273 vs 0.0075s-1, Fig.3A). PSA also reduced from 25.7 to 0.78 ng/ml. This showed early responses to treatment, whereas changes were much less discernible in T2w or DW images (Fig.3B).
A second patient had bilateral prostate cancer found at radical prostatectomy (Fig.4). HP-13C exam conducted prior to surgery enabled correlation between kPL maps and pathological findings. Regions of the highest kPL (red and bright orange) were associated with Gleason 4+3 cancer. Regions with relatively lower kPL values (blue to purple) correlated with Gleason 3+4 and 3+3 cancer.
A third patient had extensive castration-resistant prostate cancer (Gleason 4+5). One month after the initiation of ADT (Zytiga), high kPL was observed at HP-13C exam (Fig.5), associated with PSA increase from 15.8 to 20 ng/ml.
In this study the combination of HP-13C MRI and kinetic models enabled quantitative detection of prostate cancer metabolism in patients. The study results support a role for HP-13C MRI in the assessment of prostate cancer aggressiveness and treatment response to address current unmet clinical needs.
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