The measurement of R1rho (1/T1rho) spectrum and its asymmetry have several advantages over Chemical Exchange Saturation Transfer (CEST) to probe chemical exchange effect. However, these approaches suffer from B1 Radiofrequency (RF) and B0 field inhomogeneities. In this work, we proposed a new approach to perform robust R1rho asymmetry measurement using adiabatic spin-lock RF pulse and demonstrated its potential to probe metabolites.
We used a toggling inversion approach reported,1 and combine it with the adiabatic spin-lock approach3,4 to address the aforementioned problem. The proposed spin-lock RF pulse cluster is shown in Figure 1. A toggling inversion pulse and crushers are applied preceding off-resonance adiabatic spin-lock. When the inversion pulse is turned off, the magnetization after spin-lock can be expressed as:$$M^{tsl}=M_{01}\cdot e^{-R_{1\rho }\cdot tsl}+M_{01}S_{ss}\cdot (1-e^{-R_{1\rho }\cdot tsl}), [1]$$and when the inversion pulse is turned on, the magnetization can be expressed as:$$M_{i}^{tsl}=-M_{02}\cdot e^{-R_{1\rho }\cdot tsl}+M_{02}S_{ss}\cdot (1-e^{-R_{1\rho }\cdot tsl}), [2]$$where $$$M_{01}$$$ and $$$M_{02}$$$ are the magnetizations when TSL = 0ms, $$$S_{ss}$$$ is the steady state signal. Note that $$$M_{01}$$$ and $$$M_{02}$$$ are different at the presence of field inhomogeneities. Therefore, it is not possible to remove them by subtracting the two equations. To address this, two additional pairs of data at TSL 0ms are collected to remove $$$M_{01}$$$ and $$$M_{02}$$$. After this process, the R1rho-spectrum can then be calculated from the difference of the magnetization with and without the inversion RF pulse. The R1rho asymmetry at the chemical shift of the metabolites can be calculated from the R1rho-spectrum.
We performed the conventional approach1 and our proposed approach using simulation, phantom and in vivo experiments. Simulations were performed using parameters of cartilage, five concentrations of metabolites are selected from 0 to 0.1. Three groups of B1 RF and B0 field inhomogeneities were added: control (no B1 RF and B0 inhomogeneity), moderate (90% B1 and 50Hz B0) and severe (80% B1 and -100Hz B0). Six tubes of 4% agarose and myo-inositol concentration 0mM, 50mM, 100mM, 150mM, 200mM and 300mM were used in the phantom study. Phantoms and in vivo knee data sets were acquired from a Philips Achieva TX 3.0T system using eight-channel head and knee coils, respectively. Volunteer scan was conducted under the approval of the Institutional Review. 2D Fast Spin Echo was used for imaging data acquisition. Scans were performed at resonance frequency offsets (FO) from -300 to 300Hz with 25Hz increment, the same frequency offset was used to run simulations, and repeated with 2Hz increment. Frequencies of spin-lock (FSL) for simulations and phantoms were 150Hz, 200Hz and 300Hz, for in vivo were 150Hz and 250Hz. Time of spin-lock was 60ms. For Phantom and in vivo experiments, an order of 15 polynomial fitting was used to fit the R1rho-spectrum to perform asymmetry analysis. R1rho asymmetry was calculated at 0.9ppm to 1.1 ppm.